LIBRARY OF INSTITUTE OF ADVANCED MATERIAL STUDY, KYUSHU UNIVERSITY





The Reports of Institute of Advanced Material Study, Kyushu University

Updated on June 23, 1997



The Reports of Institute of Advanced Material Study, Kyushu University, Vol. 11, No. 2 (1997)

In Memory of Our Laboratory
Masashi Tashiro, 11-2, 57-76

Collision-Activated Dissociation Spectra for the Characterization of the Diels-Alder Adducts between C60 and Troponoids
Akira Mori, Ji-Feng Liu, Nobuo Kato, Ryuichi Isobe, and Hitoshi Takeshita, 11-2, 77-82

Photoaddition Reaction of Methyl 2,4-Dioxopentanoate with Chloroprene
Toshihide Hatsui, Tomokazu Hashiguchi, and Hitoshi Takeshita, 11-2, 83-85

Condensation of Refrigerant Mixture HCFC-123/HFC-134a on a Staggered Bundle of Horizontal Finned Tubes
Hiroshi Honda, Hiroshi Takamatsu, and Nobuo Takata, 11-2, 87-94

A Consideration of the Morphology of Electrochemically Deposited Lithium
Jun-ichi Yamaki, 11-2, 95-98

Thermal CVD of Silica thin film by Organic Silan Compound Byunghoon Kim, Ryoma Okazaki, Yasunobu Akiyama, Tsuneyuki Sato, and Nobuyuki Imaishi , 11-2, 99-103

Synthesis, Structures and Inclusion Properties of [(Arenylaminocarbonyl)methoxy]hexahomotrioxacalix[3]arenes
Takehiko Yamato and Fenglei Zhang, 11-2, 105-112

Prediction Method of In-tube Condensation of Multi-component Vapor Mixture
Shigeru Koyama and Sang-Mu Lee, 11-2, 113-119

Deuterium Labelling of L-Tyrosine with Raney Alloys in Alkaline Deuterium Oxide Solutions
Tsusuki Hirohisa, Mukumoto Mamoru, Udagawa Jun, Mataka Shuntaro, and Tashiro Masashi, 11-2, 121-124

Synthesis of 2-Aminomethyl-5-tert-butylphenols
Gouki Fukata, Tadanori Kanai, and Shuntaro Mataka, 11-2, 125-129

Preparation and Conformational Behavior of Trimethoxy[2.2.3]metacyclophanes
Tsuyoshi Sawada, Takehito Tsukinoki, Masashi Tashiro, and Shuntaro Mataka, 11-2, 131-134

Computational Studies on Intramolecular Cation/p Interactions in 8-Bromomethyl[2.2]metacyclophane Derivatives
Kan Tanaka, Takaaki Sonoda, and Shuntaro Mataka , 11-2, 135-140

Numerical Analyses for Two-Phase Flow in a Vertical Cylinder
Sunao Kusu, Kenya Kuwagi, and Hiroyuki Ozoe, 11-2, 141-145

Chiral Building Blocks from (+)-(S)-7,7a-Dihydro-7a-methylindane-1,5(6H)-dione (Hajos-Parrish Diketone)
Thies Thiemann, Michael Noltemeyer, and Armin de Meijere, 11-2, 147-152

Estimation of Through-space Interaction between Two Aromatic Ringsin Metacyclophanes
Akihiko Tsuge and Tetsuji Moriguchi, 11-2, 153-158

Study on Ionization and Dissociation Processes of Plasma Processing Gases Using a Thermal-Energy Ion-Beam Method
Masaharu Tsuji and Yukio Nishimura, 11-2, 159-168

Soluble Polyimides with Aliphatic Structure
Yusuke Tsuda, 11-2, 169-174

Photoreactive Dinuclear Organometallic Complexes
Hideo Nagashima, Akihiro Suzuki, 11-2, 175-180

Lanthanide-Catalyzed endo-Selective Hetero Diels-Alder Reactions of 4-Substituted Methyl (E)-2-Oxo-3-butenoates with Vinyl Ethers
Eiji Wada, Naoki Imachi, Govindaraj Kumaran, and Shuji Kanemasa, 11-2, 181-184



The Reports of Institute of Advanced Material Study, Kyushu University, Vol. 11, No. 1 (1997)

Numerical Study on Self-insulated Gas-to-gas Heat Exchanger
Toshio Tomimura, Ping Wu, Motoo Fujii, and Ryozo Echigo 11-1, 1-5

Low Pressure MOCVD of Li2O or Li2CO3 thin films from Li(DPM)
Sang-Chol Jung and Nobuyuki Imaishi 11-1, 7-12

LiNbO3 Thin Film Grown by LPMOCVD Using b-Diketonate Metal-Organic Complexes
Sang-Chol Jung and Nobuyuki Imaishi 11-1, 13-16

Development of Discharge-Flow Type of Chemical Dry Etching Apparatus
Masaharu Tsuji and Yukio Nishimura 11-1, 17-21

Titles of Publication and Presentation in 1996
Oral Presentation, 11-1, 23-42
Publication in Academic Societies, 11-1, 43-56



The Reports of Institute of Advanced Material Study, Kyushu University, Vol. 10, No. 2 (1996)

Approximate Solution for Film Condensation of Pure Refrigerant on a Finned Vertical Surface
Shigeru Koyama, Jian Yu, and Tatsuya Matsumoto 10-2, 129-136

Heat Transfer and Flow Characteristics of Pure Refrigerant HCFC123 in Falling Film Type Plate-Fin Evaporator
Shigeru Koyama, Jun'ichi Oohara, Ken Kuwahara, and Hiroyasu Nishiyama10-2, 137-144

Condensation of Pure Refrigerants in Microfin Tubes - A Correlation for Local Heat Transfer Coefficient -
Jian Yu and Shigeru Koyama 10-2, 145-150



The Reports of Institute of Advanced Material Study, Kyushu University, Vol. 10, No. 1 (1996)

Art in Organic Chemistry
Hitoshi Takeshita 10-1, 1-8

Acid-Catalyzed Rearrangement of Tropone Endoperoxides. An 8,9-Dioxabicyclo[3.2.2]nona- 3,6-diene Derivative to an 8-Oxabicyclo[3.2.1]octane Derivative
Akira Mori and Hitoshi Takeshita, 10-1, 9-11

Vibrational Distributions of CS+(B2S+) Produced from the Dissociative Charge-Transfer Reactions of He+ with CS2 and OCS at Thermal Energy
Masaharu Tsuji , Shin-ichi Shimada , Kazumi Mizukami, Hiroshi Obase, and Yukio Nishimura, 10-1, 13-16

Synthetic Photochemistry. LXX. Efficient Formation of An Eudesmane Skeleton by the de Mayo Reaction between 1-Isopropyl-4-methylcyclohexa-1,3-diene and Methyl 2,4-Dioxopentanoate
Narukuni Hirata, Toshihide Hatsui, Akira Mori, and Hitoshi Takeshita, 10-1, 17-21

Substituent Effects of 1,2-Bis(2thienyl)perfluorocyclopentenes
Kingo Uchida, Tadatsugu Yamaguchi, and Masahiro Irie, 10-1, 23-26

Thermolysis of Spiro[2,2-dimethylbicyclo[2.2.2]octa-5,7-diene-3,3-cyclopropene]. An Attempt to Synthesize 4,4-Dimethylmethylenecyclopropene
Akira Mori and Ramon Mosquera, 10-1, 27-29

Synthesis and Thermal Properties of Some Benzenes Incorporating a Perfluoroalkyl Chain
Hiroaki Okamoto, Hiroshi Murai, and Shunsuke Takenaka, 10-1, 31-33

Addition Reaction of 2-Pyrone-5-carboxylate with a-Terpinene. An Attempted Conversion of Monoterpene to Sesquiterpenoids
Toshihide Hatsui, Narukuni Hirata, and Hitoshi Takeshita, 10-1, 35-39

Estimation of Thermal Contact Conductance of Metals by Ultrasonic Waves
Toshio Tomimura, Toshihiro Kurozumi, Xing Zhang, and Motoo Fujii, 10-1, 41-44

Nafion-H Catalyzed Benzylation of Benzene and Toluene with Benzyl Alcohol
Kan Tanaka, Keiko Ishimoto, Toshio Matsuda, Shuntaro Mataka, and Masashi Tashiro, 10-1, 45-50

Preparation of 1,2-Diaminopyrene via a 1,2,5-Thiadiazole Route
Shuntaro Mataka, Yasuhiro Shidahara, Tadashi Yonemitsu, Tsuyoshi Sawada, Kazufumi Takahashi, Tori-i Akiyoshi, and Masashi Tashiro, 10-1, 51-54

TiCl4-Catalyzed Competitive Benzylation of Toluene/benzene and p -Xylene/benzene with Benzyl Chloride
Ai Hiate, Kan Tanaka, Keiko Ishimoto, Toshio Matsuda, Shuntaro Mataka,and Masashi Tashiro, 10-1, 55-60

Locus of Molten Jet in the In-Rotating-Water Spinning
Hiroshi Takamatsu, Kyu-Sang Cho, and Hiroshi Honda, 10-1, 61-66

Surface Tension and Marangoni Convection of Molten NaOH
Tomoyuki Arifuku, Hirofumi Arima, Makoto Momosaki, Shoichi Yamashiro, Tsuneyuki Sato, and Nobuyuki Imaishi, 10-1, 67-75

Oxidative Coupling and Partial Oxidation of Methane over Solid Catalysts in the Presence and
Absence of Tetrachloromethane
Shigeru Sugiyama, 10-1,77-83

Synthesis and Fluorescence Properties of N -(1-Pyrenylmethyl)-18-azacrown-6 Ether
Kannji Kubo and Tadamitsu Sakurai, 10-1, 85-87

Copper(II)- or Iron(III)-Catalyzed Aldol Reactions and Michael Additions Using Silyl Enol Ethers or Silyl Ketene Acetals
Shuji Kanemasa, Sachiyo Yoshinaga, Yoichiro Shibata, Hidetoshi Yamamoto, and Eiji Wada, 10-1, 89-92

Inverse Secondary Deuterium Kinetic Isotope Effect in Diels-Alder Reaction of Orthonaphtho- [3.3]orthoanthracenophane with Maleic Anhydride
Shuntaro Mataka, Jiang Ma, Hirohisa Tsuzuki, Nishiyama Kozaburo, Thies Thiemann, and Masashi Tashiro, 10-1, 93-94

Titles of Publication and Presentation in 1995
Oral Presentation, 10-1, 95-112
Publication in Academic Societies, 10-1, 113-127



The Reports of Institute of Advanced Material Study, Kyushu University, Vol. 9, No. 2 (1995)

Boiling and Condensation of Alternative Refrigerants in a Horizontal Smooth Tube
Jian Yu, Shigeru Koyama, Hidetaka Haraguchi, Satoru Momoki,and Akira Ishibashi, 9-2, 137-154

Experimental Investigation and Numerical Simulation on Surge in a Low Specific Speedcentrifugal Blower
Ahmed Sayed Ahmed Hassan, and Hiroshi Hayami, 9-2, 155-166

High-Pressure Diels-Alder Reaction of [C60]Fullerene with Functionalized Tropone Derivatives
Ji-Feng Liu, Seiichi Tanabe, Nobuo Kato, Akira Mori, and Hitoshi Takeshita, 9-2, 167-172

Abstracts from International Seminar on Manufacturing of Advanced Materials, 9-2, 173-191



The Reports of Institute of Advanced Material Study, Kyushu University, Vol. 9, No. 1 (1995)

Basic Knowledges on Organofluorine Compounds
Hiroshi Kobayashi, 9-1, 1-6

SiCl4+(C~2T2-X~2T1,C~2T2-A~2T2) Emissions Produced from the He(23S), Ne(3P0,2)/SiCl4 Penning Ionization and Ar+(2P3/2)/SiCl4 Charge-Transfer Reaction at Thermal Energy
Masaharu Tsuji, Masafumi Nakamura, Toshinori Mizuguchi, Nobuo Kaneko, and Yukio Nishimura, 9-1, 7-12

Effect of Spinning Condition on the Shape of Metal Wire Produced by the In-Rotating-Water Spinning Method
Hiroshi Takamatsu, Kyu-Sang Cho, Hikaru Yamashiro, and Hiroshi Honda, 9-1, 13-20

One Flask Synthesis of t-2, c-3-Disubstituted 5-Oxo-r-1-cyclopentanecarboxamides by a SmI2/HMPA-Induced Stereoselective ReductiveCoupling/Dieckmann Condensation Sequence of a,b-Unsaturated Amides
Hidetoshi Yamamoto, Shigeru KOBAYASHI, and Shuji KANEMASA, 9-1, 21-26

Experimental Study of Flow Boiling Heat Transfer in a Horizontal Microfin Tube
Jian Yu, Shigeru Koyama, Satoru Momoki, 9-1, 27-42

Synthetic Photochemistry. LXIX. The Structures of the Photocycloadducts of 2-Acetoxy-4,4-dimethylbutenolide with Cyclohexene: A Revision
Toshihide Hatsui, Toshio Kitashima, and Hitoshi Takeshita, 9-1, 43-46

Synthesis, Lipophilicity, and Stability of Tetrakis(pentafluorophenyl)borate (FTPB) Anion under Highly Acidic Conditions in Comparison with Those of Tetrakis(3,5-bis(trifluoromethyl)- phenyl)borate (TFPB) Anio
Minoru Isshiki, Hiroshi Kobayashi, and Takaaki Sonoda, 9-1, 47-55

Gas Flow and Heat Transfer in a Horizontal Cold-Wall CVD Reactor -- Two and Three Dimensional Models and Flow Visualization --
Ken-ichiro Tanoue, Tsuneyuki Sato, and Nobuyuki Imaishi, 9-1, 57-67

Mean Thermal Contact Resistance of Wavy Solid Surfaces
Toshio Tomimura, Motoo Fujii, Yasunori Kawamura, Jun Sakugawa, and Toshiniro Kurozumi, 9-1, 69-73

A Numerical Analysis and Measurements of Acoustic Streaming
Yusei Izumi, Xing Zhang, and Motoo Fujii, 9-1, 69-85

Preparation and Charactarization of 10b, 10c-Dihydropyrenes
Masashi Tashiro, Shuntaro Mataka, Tsuyoshi Sawada, Keisuke Mimura, Masaki Wakabayashi, and Takehiko Yamato, 9-1, 87-93

A Formal Total Synthesis of Colchicine via the Scott's Intermediate. Palladium(0)-Mediated meta-Ethynylation of a Tropolone Derivative
Hitoshi Takeshita, Seiichi Tanabe, Ryoji Mori, and Akira Mori, 9-1, 95-98

Condensation of Polyfluoroalkanols to Tropolone to Form 2-(Polyfluoroalkoxy)tropone and Their High-Pressure Diels-Alder Reaction with [60]Fullerene
Ji-Feng Liu, Nobuo Kato, Akira Mori, Yukari Ikeda, and Hitoshi Takeshita, 9-1, 99-102

Titles of Publication and Presentation in 1994.
Oral Presentation, 9-1, 103-121
Publication in Academic Societies, 9-1, 122-135



The Reports of Institute of Advanced Material Study, Kyushu University, Vol. 8, No. 2 (1994)

Synthesis and Properties of Poly((perfluoroalkul) sulfonyl) amides and Methanide Ions as New Types of Anionic Phase-Transfer Catalysts in Azo Coupling Reactions.
Hiroshi Kobayashi, Hans-Dieter Meyer zu Duttingdodf, Jin Nie, and Takaaki Sonoda, 8-2, 231-243

Problems on Pattern Image Velocimetry
Hiroshi Hayami, Shinichiro Aramaki, ###Hitoshi Tsutsui###, and Toru Koso, 8-2, 245-251

Chemiluminescent Mechanism of Alkylacridines and Acridinium Salts.
Kuniaki Yamabe, 8-2, 253-258

Photochromic Diarylethenes for Optical Data Storage
Kingo Uchida, Masahiro Irie, 8-2, 259-264



The Reports of Institute of Advanced Material Study, Kyushu University, Vol. 8, No. 1 (1994)

My Heat Transfer Research - Its Method and Experience
Tetsu Fujii, 8-1, 1-16

Synthetic Photochemistry. LXVI. The Photoaddition of 2-Oxo-g-valerolactone to Cyclohexene.
Toshihide Hatsui, Toshio Kitashima, Hitoshi Takeshita, 8-1,17-21

Numerical Simulation of Oscillatory Axisymmetric Marangoni Convection in Small Liquid Bridge.
Shoichi Yasuhiro, Nobuyuki Imaishi, 8-1, 23-33

Generation of Pulsed Radical Beams and Thier Spectroscopic Observation.
Yukio Nishimura, Naohiko Nakano, Hiroki Ujita, and Hiroshi Sekiya, 8-1, 35-40

Deuteration of Bromophenol Derivatives with Cu-Al Alloy in a D2O Solution of Sodium Carbonate or Barium Oxide.
Takaaki Kakinami, Yukiko Iida,Shoji Kajigaeshi, Hisao Eguchi, Masashi Tashiro, 8-1,41-43

Numerical Caluculation of Transient Response of Natural Convection in a Cavity.
Hiroyuki Hirano and Hiroyuki Ozoe, 8-1, 45-52

Convection and Solidification with Applications to Crystal Glowth.
Graham de Vahl Davis, 8-1, 53-59

Condensation and Evaporation of Refrigerants in a Plate Fin Heat Exchanger.
Tomoyasu Yara, Shigeru Koyama, and Tetsu Fujii, 8-1, 61-69

Asymmetric Synthesis of 3-(1-Phenylethylamino)-1-propanol form 3-[(1-Phenylethylidene)amino]-propene by a Sequence of HydroborationªEImine Reduction.
Junji Tanaka, Hiroaki Mimaki, and Shuji Kanemasa, 8-1, 71-78

An Experiment on the Process for Producing Vapor Growth Carbon Fiber by CVD.
Noboru Fujimoto, Shigeru Koyama, and Tetsu Fujii, 8-1, 79-86

A Non-Contact Measurement of Thermal Conductivity and Diffusivity of Anisotropic Materials.
Motoo Fujii, Soochun Paku, Toshio Tomimura, and Xing Zhang, 8-1, 87-98

Simultaneous Measurements of Thermal Conductivity and Diffusivity of Liquids with a Transient Short-Hot-Wire Method.
Motoo Fujii, Xing Zhang, Seiji Fujiwara, Toshio Tomimura, and Nobuyuki Imaishi, 8-1, 99-105

Study of Bubble Nucleation using Molecular Dynamics Method.
Yasuyuki Ikegami and Takayoshi Inoue, 8-1, 107-118

Natural Convection Heat Transfer from an Array of Vertical Parallel Plates with Protruding and Discrete Heat Sources. (Prediction of Protrusiion Surface Temperature)
Motoo Fujii, Satoru Gima, Toshio Tomimura, and Xing Zhang, 8-1, 119-129

Noncontact Measurement of Internal Temperature Distribution using Ultrasonic Computed Tomography. (The 2nd Report: Numerical Simulation and Experimental Measurement)
Motoo Fujii, Xing Zhang, Tooru Kumamori, 8-1, 131-139

Effect of Basset Term on the Analysis of the Particle Motion in Oscillating Flows.
Hiromi Yamamoto, Toru Koso, Hiroshi Hayami, and Keiichirou Hirata, 8-1, 141-147

Recent Advances in Enhancing Shell-Side Condensation in Refrigerant Condensers.
Hiroshi Honda, 8-1, 149-162

Synthesis of New Troponoid Liquid Crystals
Akira Mori, 8-1, 163-174

Pattern Image Processing Measurements and Application to the Flow in a Rotating Impeller.
Hiroshi Hayami, Dexin Chen, Toru Koso, 8-1, 175-184

Synthesis and Mercurophilic Properties of Bis(2-troponyl) Thioethers of Di-, Tri-, and Tetraethylene Glycols.
Akira Mori, Kanji Kubo, Shun-ichi Hirayama, Hitoshi Takeshita, 8-1, 185-188

Organic Nonlinear Optical Materials and Organic Microcrystals.
Hachiro Nakanishi, 8-1, 189-190

Photo and Electrical Properties of Organopolysilanes and Their Applications.
Masaaki Yokoyama, 8-1, 191-193

Regulation of Liquid Crystalline Alignment by Photochemical Reaction.
Kunihiro Ichimura, 8-1, 195-196

Titles of Publication and Presentation in 1993.
Oral Presentation, 8-1, 197-213
Publication in Academic Societies, 8-1, 214-229



The Reports of Institute of Advanced Material Study, Kyushu University, Vol. 7, No. 2 (1993)

Crystallization Experiment of Molten Tin by a Czochralski Method
Mitsuo Iwamoto, Keiji Toh, Katsuhide Aikawa, and Hiroyuki Ozoe, 7-2, 151-157

Total Synthesis of Optically - Active ShizukaÃacoradienol by Means of High - Pressure Diels - Alder Reaction
Toshihide Hatsui, Tomokazu Hashiguchi, and Hitoshi Takeshita , 7-2, 159-166

The Simultaneous Measurements of Thermal Conductivity and Diffusivity with a Short-Hot-Wire
Xing Zhang, Toshio Tomimura, and Motoo Fujii, 7-2, 167-171

Measurements of Liqudi-Solid Contact and Electromotive Force during Rapid Quenching of Thin Wires in Water
Hiroshi Honda, Hiroshi Takamatsu, and Hikaru Yamashiro, 7-2, 173-180

Noncontact Measurement of Internal Temperature Distribution using Ultrasonic Computed Tomography (The 1st Report: Numerical Simulation for Estimating Measuring Accuracy)
Motoo Fujii, Xing Zhang, and Tooru Kumamori, 7-2, 181-190


Prediction of Heat Transfer Performance of Air-cooled Condensers Using Alternative Refrigerants R123 and R134a instead of R11 and R12
Tetsu Fujii, and Hidehiko Kogawa, 7-2, 191-193



The Reports of Institute of Advanced Material Study, Kyushu University, Vol. 7, No. 1 (1993)

Electronic Spectra of Jet-Cooled 3-and 4-Chlorotropolones. Influence of Asymmetric Substitution on the Intramolecular Hydrogen Bonding.
Takeshi Tsuji, Hiroshi Sekiya, Sayaka Ito, Hiroshi Ujita, Mariko Habu, Akira Mori, Hitoshi Takeshita, and Yukio Nishimura, 7-1, l-14

Heat Transfer Characteristics of a Gas-to-Gas Heat Exchanger Based on Rediative Transfer (In the Case of Relatively Low Temperatures (750-900[K]))
Toshio Tomimura, Motoo Fujii, Masahiro Kobessho, Michihiko Torio, and Ryozo Echigo, 7-1, 15-20

Natural Convection Heat Transfer from Vertical Parallel Plates to Air
Motoo Fujii, Satoru Gima, Toshio Tomimura, and Xing Zhang, 7-1, 21-27

The Total Synthesis of Optically Active DiplophyIolide A and Dip1ophy11in
Nobuo Kato, Hideyuki Nishikawa, and Hitoshi Takeshita, 7-1, 29-38

An Evaluation Method of View Factor Integral in Axisymmetric Systems
Takao Tsukada, Mitsunori Hozawa, Yuji Ohba, and Nobuyuki Imaishi, 7-1, 39-46

New Development of Organoselenium Reagents in Organic Synthesis and Its Applications to Natural Product Synthesis
Masaaki Miyashita, 7-1, 47-51

Molecular Design of Functional Polynuclear Metal Complexes
Hisashi Okawa, 7-1, 53-57

Studies on the Development of New Synthetic Reagents. Synthetic Utilization of Functionalized a , b -Unsaturated Ketones
Eiji Wada, 7-1, 59-70

Novel Reactions and Functionalization of Cyclophanes Towards New Fields of Research
Masashi Tashiro, Shuntaro Mataka, Tsuyoshi Sawada, and Takehito Tsukinoki, 7-1, 71-102

The Solution Chemistry of TFPB Salts : The Electrophilicity of Nahed Alkali Metal lons
Hiroshi Kobayashi, Kanji Fujiki, Akihisa Nagira, Jin Nie Akinari Sonoda, and Takaaki Sonoda, 7-1, 103-113

Photoaddition Reaction of Methyl 2,4-Dioxopentanoate with 1,3-Butadiene
Toshihide Hatsui, Tomokazu Hashiguchi, and Hitoshi Takeshita, 7-1, 115-118

Titles of Publication and Presentation in 1992.
Oral Presentation, 7-1, 119-134
Publication in Academic Societies, 7-1, 135-150



The Reports of Institute of Advanced Material Study, Kyushu University, Vol. 6, No. 2 (1992)

An Experiment on Condensation of Binary Vapor Mixtures inside a Vertical Smooth Tube.
Shigeru Koyama, Hidetaka Haraguchi, Tomoyasu Yara, and Tetsu Fujii, 6-2, 67-77

Heat Transfer and Pressure Drop of Single Phase Flow inside Intenally Grooved Tubes.
Shigeru Koyama, Norihiro Inoue, Satoshi Hirakuni, Ken Kuwahara, and Tetsu Fujii, 6-2, 79-86

Syntheses of Some Arylazospiropyrans
Hiroshi Kobaayshi, Akinari Sonoda, and Takaaki Sonoda, 6-2, 87-92

Mild Intramolecular Thermal Rearrangement of 2-(2-Propynylsulfinyl)tropone and Its Homologues to Cyclohepta[b]thiophen-8-ones
Bing Zhu Yin, Akira Mori, and Hitoshi Takeshita, 6-2,93-102

Natural Evaporation of a Sessile Drop on an Unheated Plate
Motoo Fujii and Toshio Tomimura, 6-2, 103-108

On the Evaluation of the Heat Transfer Coefficient inside the Inner Tube of a Double Tube Heat Exchanger (In the case of turbulent flow inside the inner tube and laminar flow in the annulus)
Satoru Momoki, Jian Yu, Shigeru Koyama, and Tetsu Fujii, 6-2, 109-114

Expressions of Thermophysical Properties of Helium and Argon
Ken Kuwahara, and Tetsu Fujii 6-2, 115-118

Reaction Conditions and Distribution of Products in Chlorination of Phenol
Akiyoshi Tori-i, Toshimi Sugita, Hisao Eguchi, Shuntaro Mataka, and Masashi Tashiro 6-2, 119-124



The Reports of Institute of Advanced Material Study, Kyushu University, Vol. 6, No. 1 (1992)

Reference Temperature for Evaluating Physical Properties of Condensate Film in the case of Free-Convection Laminar Film Condensation
Kan'ei Shinzato, Jong Boong Lee, and Tetsu Fujii, 6-1, 1-9

Synthetic Photochemistry. LIX. Intramolecular Photocycloaddition of 2(3-Butenyl)-2,6-dimethy-4H-1,3-dioxin-4-one
Ying She Cuii, Nobuo Kato, Akira Mori, Hitoshi Takeshita, and Yoshiaki Nagano, 6-1, 11-15

Natural Convection Heat Transfer from Vertical Parallel Plates to Air (Effects of Model Packages)
Motoo Fujii, Satoru Gima, Toshio Tomimura, and Xing Zhang, 6-1, 17-24

Present Status of Thin Film Technology Applied for Si ULSI and Expectation of Their Problem Solution Created by the University Researchers
Katsuro Sugawara, 6-1, 25-36

Titles of Publication and Presentation in 1991.
Oral Presentation, 6-1, 37-51
Publication in Academic Societies, 6-1, 52-66



The Reports of Institute of Advanced Material Study, Kyushu University, Vol. 5, No. 2 (1991)

Analysis of Advanced Material Processing
Nobuyuki Imaishi, Tsuneyuki Sato, and Yasunobu Akiyama, 5-2, 93-118

Recent Progress of Research in Phase Change Process
Tetsu Fujii, Shigeru Koyama, Kan'ei Shinzato, and Tomoyasu Yara, 5-2, 119-123

Development of a Vapor Compression Heat Pump System Using Non-azeotropic Refrigerant Mixtures
Tetsu Fujii, Shigeru Koyama, Hiroshi Takamatsu, Kan'ei Shinzato, and Tomoyasu Yara, 5-2, 125-137

Heat Transfer Characteristics During Rapid Quenching of a Thin Wire
Hiroshi Honda, Hiroshi Takamatsu, Hikaru Yamashiro, and Nobuo Takada, 5-2, 139-145

Augmentation of Condensation Heat Transfer by Finning of Tubes
Hiroshi Honda, Hiroshi Takamatsu, and Nobuo Takada, 5-2, 147-164

Research and Development of Freon Transonic Turbo Compressor
Hiroshi Hayami, Toru Koso, and Nobumasa Kawaguchi, 5-2, 165-173

Study on the Nature of Turbulent Intermittency in a Coflowing Turbulent Free Jet
Toru Koso and Hiroshi Hayami, 5-2, 175-188

Combined Convection Heat Transfer with Conduction and Radiation
Motoo Fujii, Toshio Tomimura, and Xing Zhang, 5-2, 189-200

Representative Viscosity of Condensate in the Case of Laminar Forced-Convection Condensation of Pure Vapors.
Tetsu Fujii, Jong Boong Lee, and Kan'ei Shinzato, 5-2, 201-207

Representative Physical Properties of Condensate in the Case of Laminar Forced-Convection Condensation of Pure Vapors.
Tetsu Fujii, Jong Boong Lee, and Kan'ei Shinzato, 5-2, 209-213

Representative Physical Properties for the Vapor Boundary Layer in the Case of Laminar Film Condensation of Binary Vapor Mixtures. ( I ) Forced-Convection Condensation
Tetsu Fujii, Jong Boong Lee, Kan'ei Shinzato, and Masaharu Watabe, 5-2, 215-221

Representative Physical Properties for the Vapor Boundary Layer in the Case of Laminar Film Condensation of Binary Vapor Mixtures. (II) Free-Convection Condensation
Tetsu Fujii, Jong Boong Lee, Kan'ei Shinzato, and Masaharu Watabe, 5-2, 223-228

The Reports of Institute of Advanced Material Study, Kyushu University, Vol. 5, No. 1 (1991)

The High-Pressure Cycloadditions of Tropone to Styrenes. Predominant Formation of [8+2] Cycloadducts from q-Methylstyrene
Zhi-Hong Li, Akira Mori, and Hitoshi Takeshita, 5-1, l-9

Stusy on ab initio Calculation Method of Thermal and Fluid Properties
Susumu Kotake, 5-1, l1-19

Fast Formation of Insulating Oxide Thin Films by Excimer-Laser-Induced CVD Methods. Masaharu Tsuji, 5-1, 20-31

Atomic and Molecular Clusters : Review of the Studies
Susumu Kotake, 5-1, 33-62

Intramolecular Disproportionation Reactions of 4, 6-Bis (chloromethyl -2, 5-dimethoxytropone via Heptafulvene Intermediates
Shun-ichi Hirayama, Akira Mori, and Hitoshi Takeshita, 5-1, 63-65
Titles of Publication and Presentation in 1990.
Oral Presentation, 5-1, 67-78
Publication in Academic Societies, 5-1, 79-91



The Reports of Institute of Advanced Material Study, Kyushu University, Vol. 4, No. 2 (1990)

Study on Coal Liquefaction and Petroleum Refining Processes
Isao Mochida, Kinya Sakanishi, and Ryuji Sakata, 4-2, 69-73

Development of Novel Catalysts and Adsorbents for Environmental Protection
Isao Mochida, Shizuo Kawano, and Seiki Kisamori, 4-2, 75-80

Control of Texture in Carbon Materials
Isao Mochida, and Yozo Korai, 4-2, 81-88

Dissociation of the Group IV Compounds by Collisions with Metastable Rare-Gas Atoms.
Yukio Nishimura, Masaharu Tsuji, and Hiroshi Sekiya, 4-2, 89-96

Photo-induced Intramolecular Proton Transfer and Its Application
Yukio Nishimura, and Hiroshi Sekiya, 4-2, 97-105

Materials for Molecular Photonics
Masahiro Irie, Kingo Uchida, and Norihisa Tanio, 4-2, 107-113

Numerical Analyses and Experiments of Transport Processes
Hiroyuki Ozoe, Takayoshi Inoue, and Mitsuo Iwanoto, 4-2, 115-149

The13CNMRChemical Shift Comparisons of Dihydrohomobarrelenones
Zhiª]Hong Li, Nobuo Kato, Akira Mori, and Hitoshi Takeshita, 4-2, 151-156

Synthesis and Characterization of New TrinuclearlRhªiIªjª]Imidazolate Complexes
Noriaki Kihara, Kenji Saeki, and Masashi Tashiro, 4-2, 157-161

Optical Spectroscopic Studies on Penning Ionization and Chargeª]Transfer Reactionsat Thermal Energy by Using FIowing Afterglow
Masaharu Tsuji, and Yukio Nishimura, 4-2, 163-174

Langmuir-Blodgett k Films and Molecular Devices
Michio Sugi, 4-2, 175-188

Chemical Aspects of High Temperature Superconductors
Shin-Pei Matsuda, 4-2, 189-195

Photoaddition Reaction of5ªC5Dimethylcyclohexaneª]1ªC3ª]dione with Quadricyclane
Toshihide Hatsui, Koichi Hayashi, and Hitoshi Takeshita, 4-2, 197-200

Highª]Pressure Dielsª]Alder Reaction of Tropone Acetal with Several Dienophiles
Zhiª|Hong Li, Akira Mori, Hitoshi Takeshita, and Yoshiaki Nagano, 4-2, 201-204



The Reports of Institute of Advanced Material Study, Kyushu University, Vol. 4, No. 1 (1990)

Comparison of Equations of State for Estimating Thermodynamic Properties of Pure R22, Pure R114 and Their Mixtures.
Hiroshi Takamatsu, and Yasuyuki Ikegami, 4-1, 1-14

A Numerical Analysis of Laminar Mixed Convection Heat Transfer between Vertical Parallel Plates with Discrete sources Heated at Different Rate (Part 2:Conducting Plaes).
Toshio Tomimura, and Motoo Fujii, 4-1, 15-22

Program Package for Thermophysical Properties of Binary Mixtures by the BWR Equation of State
Hiroshi Takamatsu, and Yasuyuki Ikegami, 4-1, 23-37

Program Package for Thermophysical Properties of Binary Mixtures by the SRK Equation of State
Hiroshi Takamatsu, and Yasuyuki Ikegami, 4-1, 39-46

Titles of Publication and Presentation in 1990.
Oral Presentation, 4-1, 47-57
Publication in Academic Societies, 4-1, 58-67



The Reports of Institute of Advanced Material Study, Kyushu University, Vol. 3, No. 2 (1990)

New Synthetic Methodologies Developed in the Institute
Shuij Kanemasa, Eiij Wada, and JunjjTanaka, 3-2, 79-106

Structural Design and Syntheses of Functional Molecules
Masashi Tashiro, Shuntaro Mataka, Akihiko Tsuge, and Hirohisa Tsuzuki, 3-2, 107-131

Utility of Organic Fluorine Compounds in Molecular Designing of Functional Material
Junij Ichikawa, Hiroshi Kobayashi, and Takaaki Sonoda, 3-2, 133-144

Recent Progress in the Functional Material Syntheses from Novel Aromatic Compounds. Hitoshi Takeshita, Akira Mori, and Tomohiro Nagao, 3-2, 145-166

A New Methodology for Stereocontrolled Carbon-Cafbon Bond Formation. Frontier Orbital- and Chelation-Contfolled Diastereoselective Michael Additions of a-Amino Esters Leading to Unnatural Amino Acid Derivatives.
Shuji Kanemasa, 3-2, 167-180

Preparation and Conformation o f Metacyclophanes Having Three and Four Benzene Rings.
Shuntaro Mataka, Akihiko Tsuge, and Masashi Tashiro, 3-2, 181-191

Total Synthesis of Biologically-active Terpenoids
Nobuo Kato, 3-2, 193-203

Molecular Design for Higher-Order Functions. Novel Catalytic Functions Caused by High Lipophilicity of Polyiluorinated Tetraphenylboron Ate-Complexes
Hiroshi Kobayashi, 3-2, 205-216

Molecular Design for Controlling Functlonality-Photochemical Properties of Ordered Chromophores in Monolayer Assemblies
Toshihiko Nagamura, 3-2, 217-227

Application of Molecular Mechanics Calculations to Some Organic Reactions
Yoshimasa Fukazawa, 3-2, 229-234



The Reports of Institute of Advanced Material Study, Kyushu University, Vol. 3, No. 1 (1989)

Synthesis of Bis (silyloxy) Cross-Conjugated Polyenes and Their Sequential Ring Formations via Electrocyclization
Eiji Wada, Shuji Kanemasa, Nobuo Kimura, Hirohiko Kimura, and Otohiko Tsuge, 3-1, 1-8

Numerical Analysis of Velocity, Terhperature and Thermal Stress Fields in Czochralski Furnace
Nobuyuki Imaishi, Takao Tsukada, and Mitsunori Hozawa, 3-1, 9-19

Experimental Study of the Enhancement of Condensation Heat Transfer on Downward-Facing Horizontal Surfaces
Hiroshi Honda, Shigeru, Nozu, and Bunken Uchima, 3-1, 21-32

Natural Convection Heat Transfer in Enclosed Horizontal Fluid Layer Heated Below
Kiyoji Miyabe, and Motoo Fujii 3-1, 33-45

Metacyclophanes and Related Compounds. XXV. Generation of Bis (o-quinone methide) from [2.2]Metacyclophane Having Spiro Skeleton and Its Reactions with Alcohols, Acetic Acid, and Ethenes
Takehiko Yamato, Masami Kajihara , Jun-ichi Matsumoto, Akiyoshi Torii, and Masashi Tashiro, 3-1, 47-53

The Reduction of I ,2-Dioxetanes to cis-1,2-Diols by Superoxide. The Mechanism of the Process found in the Rose Bengal-Sensitized Photooxygenation
Toshihide Hatsui, and Hitoshi Takeshita, 3-1, 55-57

Titles of Publication and Presentation in 1988.
Oral Presentation, 3-1, 59-68
Publication in Academic Societies, 3-1, 69-78



The Reports of Institute of Advanced Material Study, Kyushu University, Vol. 2, No. 2 (1988)

Enviromental Impacts of Coal Mining and Preventive Measures in Japan
Kazuo Aoki, Tetsuro Esaki, Tsuyoshi Kimura, Nobuhiro Kameda, and Tadashi Nishida, 2-2, 231-240

Synthetic Photochemistry. XLVIII. Stereocontrolled Generation of the Ophiobolane Type 5-8-5-Membered Tricyclic Ring System
Nobuo Kato, Shoji Ohbuchi, and Hitoshi Takeshita, 2-2, 241-251

Control of Skin-Core Structure in Mesophase Pitch Based Carbon Fiber (1) Introduction of Skin-Core Structure in the Thin Fiber and Carbonization under Strain
Isao Mochida, Shu Ming Zeng, Yozo Korai, and Tadayuki Matsumoto, 2-2, 253-260

Reduction of Unsaturated Aliphatic Mono- and Dicarboxylic Acids and Brominated Aliphatic Acids with Raney Alloys in an Alkaline Solution, Affording the Corresponding Saturated Aliphatic Acids
Masashi Tashiro, Shuntaro Mataka, Hirohisa Tsuzuki, Shoji Ogasahara, Shin-ichiro Isobe, and Tadashi Yonemistu, 2-2, 261-268

Electrochemical Oxidation of 5-Hydroxytropolone
Akira Mori, Hiroyasu Watanabe, and Hitoshi Takeshita, 2-2, 269-273

Heat Transfer Characteristics of Freon Gas (Rll4) in a Rectangular Square
Separated by a Vertical Partition
Tetsu Fujii, Shigeru Koyama, and Byung-Duck Park, 2-2, 275-285

Numerical Computation for Molecular Energy Transfer in a Thin Film
Toshio Tomimura, Hiroyuki Ozoe, and Susumu Kotake, 2-2, 287-294

Study on Natural Air Cooling of an IC Board
Motoo Fujii, and Toshio Tomimura, 2-2, 295-303



The Reports of Institute of Advanced Material Study, Kyushu University, Vol. 2, No. 1 (1988)

Research on the Heterocyclic Chemistry - Forty Years in Kyushu University.
Otohiko Tsuge, 2-1, 1-28

Quasiclassical Trajectory Calculation of the Reaction O(3P) +HI- OH(X)+I
Nobuaki Nishiyama, Hiroshi Sekiya, and Yuhio Nishimura, 2-1, 29-34

Ring-opening Reaction of 6, 8-Di-t-butyl-1,2,3,4,-tetrahydr0-9aH-pyrido [2, 1-b]-benzoxazole
Gouki Fukata, Shuntaro Mataka, and Masashi Tashiro, 2-1, 35-39

Synthetic Approaches to Cyclopropyl Phosphorylmethyl Ketones and l-Alkenyl Cyclopropyl Ketones
Otohiko Tsuge, Shuji Kanemasa, and Tatsuya Otsuka, 2-1, 41-52

Effective Energy Conversion Method between Gas Enthalpy and Thermal Radiation (Effects of Gaseous Radiation and Incoming Radiations)
Ryozo Echigo, Toshio Tomimura, Yoshio Yoshizawa, and Hidenobu Jinnouchi 2-1, 53-66

An Experimental Method to Mesure Local Heat Transfer Coefficient from a Distance
Motoo Fujii, Nelson Mugabi, Chouiku Yoshizawa, and Tetsu Fujii, 2-1, 67-78

Regioselective Preparation of Aminomethylphenols by Reduction of Mannich Bases of Halophenols with Raney Cu-AI Alloy in 10% Aqueous Sodium Hydroxide
Masashi Tashiro, Katsunori Saeki, Hirohisa Tsuzuki, Shantaro Mataka. Taizo Hatta, and Tadashi Yinemitsu, 2-1, 79-85

Bromination of Alkenes and Related Compounds by Use of Bonzyltrimethylammonium Tribromide in Aprotic and Protic Solvents
Shoji Kajigaeshi, Takaaki Kakinami, Masayuhi Moriwaki, Shizuo Fujisaki, and Masashi Tashiro, 2-1, 87 -94

Cycloaddition-Cycloreversion Sequence for One-pot Preparation of Dibenzobarfelene and Janusene Deriuatives from Anthracenes and 2, 3-Bis ( methoxycarbonyl ) -7-0xanorbornadiene
Guan Rong Tian, Akira Mori, Shigeru Sugiyama, and Hitoshi Takeshita, 2-1, 95-99

A Flowing Afterglow Study of Penning lonization Ne(3 P0,2)+ COŮC0+(A2Pi)+Ne+e-
Masaharu Tsuji, Hiroshi Obase, and Yuhio Nishimura 2-1, 101-104

Catalytic Oligomerization of Isoprene in Solution. Coordination Features of Phosphorus Ligands in the Ni (0) Complexes
Hiroshi Fujitsu, Masahiro Jono, Hidenori Okamoto, Kenjiro Takeshita, and Isao Mochida, 2-1, 105-113

Synthetic Photochemistry. XLIII. Chromium(II) Chloride-Mediated Reductive Condensations of (3S) -and (3R) -1-Iriden- 7-als with (3S)-7-Chloro-1-iridenes. 1H NMR Spectral Differentiation of the Stereochemistry
Nobuo Kato, Xue Wu, Shoji Ohbuchi, Hiroyuki Miyagawa, Shinya Tanaka, Hideo Kataoka, Takayuki Imaoka, and Hitoshi Takeshita, 2-1, 115-123

Application of a Laser Doppler Anemometer to the Study on the Nature of Turbulent Intermittency.
Toru Koso, Yutaro Nishino and Yasutoshi Senoo, 2-1, 125-142

Numerical Computation of Czochralski Mixed Convection for Molten Silicon
Hiroyuki Ozoe and Toshio Mztsui, 2-1, 143-148

The Chemistry of Azomethine Ylides Developed in the Institute
Shuji Kanemasa, 2-1, 149-177

Synthesis and Electrochemical Properties of Substituted p -Tropoquinones
Akira Mori, 2-1, 179-184

Chemistry of Trioxanes
Toshihide Hatsui, 2-1, 185-188

Fluorinated Tetraarylborates as Anionic Phase-transfer Catalysts: An Example of Molecular Design of Functional Fluoroaromatics
Junji Ichikawa, Hiroshi Kobayashi, and Tahaaki Sonoda, 2-1, 189-207

Titles of Publication and Presentation in 1987.
Oral Presentation, 2-1, 209-217
Publication in Academic Societies, 2-1, 218-229



The Reports of Institute of Advanced Material Study, Kyushu University, Vol. 1, No. 1 (1987)

Metacyclophanes and Related Compounds. 20. Reaction of Methyl [2.2] metacyclophanes with N -Bromosuccineimide
Masashi Tashiro, Takehiko Yamato, and Takashi Arimura, 1-1, 1-10

Some Lipophilic Pyridylpyridinium Tetrakis [3,5-bis(trifluoromethyl)phenyl] borates as the Catalytic Electron Mediators
Tomonobu Shimizu, Keisuke Takuma, Takaaki Sonoda, and Hiroshi Kobayashi, 1-1, 11-19

Synthesis of Bis (2,6-dihydroxy-5-oxo-1,3,6-cycloheptatrienyl)-methane from 2-Alkoxy-5-hydroxytropones and the Electrochemical Properties of Bis (3,4,7-trioxo-1,5- cycloheptadienyl)-methane Derivatives
Akira Mori, Yasutomo Goto, and Hitoshi Takeshita, 1-1, 21-27

Synthesis of 4,6-Dicyano-2,5-dimethoxytropone
Hitoshi Takeshita, Akira Mori and Shun-ichi Hirayama, 1-1, 29-33

A Flowing Afterglow Study of the Reaction C2+NOª¬CN (B2á+, A2P)+CO
Nobuaki Nishiyama, Hiroshi Sekiya, Masaharu Tsuji, and Yukio Nishimura, 1-1, 35-50

15N2+ (D'2Pgr-A2Pui) Emission Resulting from the He+ + 15N2 Charge Transfer Reaction
Hiroshi Sekiya, Masaharu Tsuji, and Yukio Nishimura, 1-1, 51-56

Condensation and Evaporation of Non-azeotropic Refrigerant Mixtures of R22 and R114 inside a Spirally Grooved Horizontal Tube
Shigeru Koyama, Akio Miyara, Hiroshi Takamatsu, Kazuo Yonemoto and Tetsu Fujii, 1-1, 57-75

Laminar Film Condensation of Multicomponent Mixtures on a Flat Plate (First Report, Forced Convection Condensation)
Shigeru Koyama, Masao Goto, and Tetsu Fujii, 1-1, 77-83

Laminer Film Condensation of Multicomponent Mixtures on a Flat Plate (Second Report, Gravity Controlled Condensation)
Shigeru Koyama, Masao Goto, Masaharu Watabe, and Tetsu Fujii, 1-1, 85-89


Test Facility and the Available Inlet Flow Condition to Transonic Radial Diffusers
Hiroshi Hayami, Yasutoshi Senoo, Kohji Nakashima, and Nobumasa Kawaguchi, 1-1, 91-96

Catalitic Activity of PAN-ACF and its Activated Form with Sulfuric Acid for the Removal of NOx
Hiroshi Fujitsu and Isao Mochida, 1-1, 97-109

Evacuation at Elevated Temperatures to Enhance the Catalytic Activity of RhªETiO2 for the Hydrogenation of CO
Nobuhide Ikeyama, Hideo Ishibashi, Hiroshi Fujitsu, and Isao Mochida, 1-1, 111-114

Titles of Publication and Presentation in 1986.
Oral Presentation, 1-1, 115-123
Publication in Academic Societies, 1-1, 124-132